Target-triggered cascade assembly of a catalytic network as an artificial enzyme for highly efficient sensing

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Target-triggered cascade assembly of a catalytic network as an artificial enzyme for highly efficient sensing.

Determining the catalytic activity of artificial enzymes is an ongoing challenge. In this work, we design a porphyrin-based enzymatic network through the target-triggered cascade assembly of catalytic nanoparticles. The nanoparticles are synthesized via the covalent binding of hemin to amino-coated gold nanoparticles and then the axial coordination of the Fe center with a dual-functional imidaz...

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Target-triggered cascade assembly of a catalytic network as an artificial enzyme for highly efficient sensing† †Electronic supplementary information (ESI) available: Experimental details, and supporting figures and tables. See DOI: 10.1039/c7sc01453h Click here for additional data file.

Determining the catalytic activity of artificial enzymes is an ongoing challenge. In this work, we design a porphyrin-based enzymatic network through the target-triggered cascade assembly of catalytic nanoparticles. The nanoparticles are synthesized via the covalent binding of hemin to amino-coated gold nanoparticles and then the axial coordination of the Fe center with a dual-functional imidaz...

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ژورنال

عنوان ژورنال: Chemical Science

سال: 2017

ISSN: 2041-6520,2041-6539

DOI: 10.1039/c7sc01453h